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× 2024 Journal Articles Linear, Y- and Ψ-shaped poly(2-(dimethylamino)ethyl methacrylate) and poly(methyl methacrylate) brushes prepared by surface-initiated polymerization from a homologous series of ATRP initiators S. Sant ; H-A. Klok
European Polymer Journal . 2024-01-13. Vol. 205 , p. 112706. DOI : 10.1016/j.eurpolymj.2023.112706. 2023 Journal Articles Supramolecular Polymer Brushes Grown by Surface-Initiated Atom Transfer Radical Polymerization from Cucurbit[7]uril-based Non-Covalent Initiators F. K. Metze ; I. Filipucci ; H-A. Klok
Angewandte Chemie-International Edition . 2023-07-17. Vol. 62 , num. 34 , p. e202305930. DOI : 10.1002/anie.202305930. Fluorinated Poly(aryl piperidinium) Membranes for Anion Exchange Membrane Fuel Cells X. Wu ; N. Chen ; C. Hu ; H-A. Klok ; Y. M. Lee et al.
Advanced Materials . 2023-05-11. Vol. 35 , num. 26 , p. 2210432. DOI : 10.1002/adma.202210432. Supramolecular Polymer Brushes F. K. Metze ; H. -A. Klok
Acs Polymers Au . 2023-02-08. DOI : 10.1021/acspolymersau.2c00067. Opportunities and Challenges for Lignin Valorization in Food Packaging, Antimicrobial, and Agricultural Applications A. Boarino ; H-A. Klok
Biomacromolecules . 2023-02-06. DOI : 10.1021/acs.biomac.2c01385. 2022 Journal Articles Uniformly Dispersed Poly(lactic acid)-Grafted Lignin Nanoparticles Enhance Antioxidant Activity and UV-Barrier Properties of Poly(lactic acid) Packaging Films A. Boarino ; A. Schreier ; Y. Leterrier ; H-A. Klok
Acs Applied Polymer Materials . 2022-05-24. DOI : 10.1021/acsapm.2c00420. Macromolecular engineering via polyhomologation F. Li ; H-A. Klok
European Polymer Journal . 2022-05-15. Vol. 171 , p. 111195. DOI : 10.1016/j.eurpolymj.2022.111195. 2021 Journal Articles Branched Poly(Aryl Piperidinium) Membranes for Anion-Exchange Membrane Fuel Cells X. Wu ; N. Chen ; H-A. Klok ; Y. M. Lee ; X. Hu
Angewandte Chemie-International Edition . 2021-12-27. p. e202114892. DOI : 10.1002/anie.202114892. Reduction-Sensitive Protein Nanogels Enhance Uptake of Model and Tumor Lysate Antigens In Vitro by Mouse- and Human-Derived Dendritic Cells C. Berti ; A. Boarino ; M. Graciotti ; L. P. E. Bader ; L. E. Kandalaft et al.
Acs Applied Bio Materials . 2021-12-20. Vol. 4 , num. 12 , p. 8291-8300. DOI : 10.1021/acsabm.1c00828. Polymethylene Brushes via Surface-Initiated C1 Polyhomologation F. Li ; S. Thiele ; H-A. Klok
Journal Of The American Chemical Society . 2021-12-01. Vol. 143 , num. 47 , p. 19873-19880. DOI : 10.1021/jacs.1c09187. Succinimidyl Carbonate-Based Amine-Reactive Polymer Brushes: Facile Fabrication of Functional Interfaces T. N. Gevrek ; A. Degirmenci ; R. Sanyal ; H-A. Klok ; A. Sanyal
Acs Applied Polymer Materials . 2021-05-14. Vol. 3 , num. 5 , p. 2507-2517. DOI : 10.1021/acsapm.1c00107. Self-assembly of protein-polymer conjugates for drug delivery C. A. Stevens ; K. Kaur ; H-A. Klok
Advanced Drug Delivery Reviews . 2021-05-11. Vol. 174 , p. 447-460. DOI : 10.1016/j.addr.2021.05.002. Biotin-NeutrAvidin Mediated Immobilization of Polymer Micro- and Nanoparticles on T Lymphocytes M. Ayer ; O. Burri ; R. Guiet ; A. Seitz ; E. Kaba et al.
Bioconjugate Chemistry . 2021-03-17. Vol. 32 , num. 3 , p. 541-552. DOI : 10.1021/acs.bioconjchem.1c00026. Structural Basis of Ligand Selectivity by a Bacterial Adhesin Lectin Involved in Multispecies Biofilm Formation S. Guo ; T. D. R. Vance ; H. Zahiri ; R. Eves ; C. A. Stevens et al.
Mbio . 2021-04-01. Vol. 12 , num. 2 , p. e00130-21. DOI : 10.1128/mBio.00130-21. Fluorescence-Based and Fluorescent Label-Free Characterization of Polymer Nanoparticle Decorated T Cells T. Thomsen ; A. B. Ayoub ; D. Psaltis ; H-A. Klok
Biomacromolecules . 2021-01-01. Vol. 22 , num. 1 , p. 190-200. DOI : 10.1021/acs.biomac.0c00969. 2020 Journal Articles T Cell-Mediated Transport of Polymer Nanoparticles across the Blood-Brain Barrier M. Ayer ; M. Schuster ; I. Gruber ; C. Blatti ; E. Kaba et al.
Advanced Healthcare Materials . 2020-11-25. p. 2001375. DOI : 10.1002/adhm.202001375. Reversibly Cross-Linking Polymer Brushes Using Interchain Disulfide Bonds P. Mocny ; H-A. Klok
Macromolecules . 2020-01-28. Vol. 53 , num. 231 , p. 731-740. DOI : 10.1021/acs.macromol.9b02199. 2019 Journal Articles Synthesis of Loop Poly(Methyl Methacrylate) Brushes via Chain-End Postpolymerization Modification P. Mocny ; M. Menetrey ; H-A. Klok
Macromolecules . 2019-11-12. Vol. 52 , num. 21 , p. 8394-8403. DOI : 10.1021/acs.macromol.9b01527. Mechanoresponsive Micro- and Nanoparticles F. K. Metze ; H-A. Klok
Chimia . 2019-02-01. Vol. 73 , num. 1 , p. 35-38. DOI : 10.2533/chimia.2019.35. Polymer brush interfaces for protein biosensing prepared by surface-initiated controlled radical polymerization M. Badoux ; M. Billing ; H-A. Klok
Polymer Chemistry . 2019. Vol. 10 , num. 23 , p. 2925-2951. DOI : 10.1039/C9PY00163H. Swelling-Induced Chain Stretching Enhances Hydrolytic Degrafting of Hydrophobic Polymer Brushes in Organic Media J. Wang ; H-A. Klok
Angewandte Chemie International Edition . 2019. Vol. 58 , p. 1-6. DOI : 10.1002/anie.201904436. Cellular Uptake and Intracellular Trafficking of Poly(N-(2-Hydroxypropyl) Methacrylamide) C. Battistella ; R. Guiet ; O. Burri ; A. Seitz ; S. Escrig et al.
Biomacromolecules . 2019. Vol. 20 , num. 1 , p. 231-242. DOI : 10.1021/acs.biomac.8b01372. 2018 Journal Articles Synthesis and Postpolymerization Modification of Fluorine-End-Labeled Poly(Pentafluorophenyl Methacrylate) Obtained via RAFT Polymerization C. Battistella ; Y. Yang ; J. Chen ; H-A. Klok
Acs Omega . 2018-08-01. Vol. 3 , num. 8 , p. 9710-9721. DOI : 10.1021/acsomega.8b01654. Stimuli-Sensitive and -Responsive Polymer Biomaterials T. W. J. Steele ; H-A. Klok
Biomacromolecules . 2018-05-01. Vol. 19 , num. 5 , p. 1375-1377. DOI : 10.1021/acs.biomac.8b00145. Polymer-Brush-Templated Three-Dimensional Molybdenum Sulfide Catalyst for Hydrogen Evolution L-A. Stern ; P. Mocny ; H. Vrubel ; T. Bilgic ; H-A. Klok et al.
ACS Applied Materials & Interfaces . 2018. Vol. 10 , num. 7 , p. 6253-6261. DOI : 10.1021/acsami.7b16679. Structure and functionality of polyelectrolyte brushes, a surface force perspective X. Xu ; M. Billing ; M. Ruths ; H-A. Klok ; J. Yu
Chemistry – An Asian Journal . 2018-08-06. Vol. 13 , num. 22 , p. 3411-3436. DOI : 10.1002/asia.201800920. pH-Sensitive Coiled-Coil Peptide-Cross-Linked Hyaluronic Acid Nanogels: Synthesis and Targeted Intracellular Protein Delivery to CD44 Positive Cancer Cells L. Ding ; Y. Jiang ; J. Zhang ; H-A. Klok ; Z. Zhong
Biomacromolecules . 2018-02-01. Vol. 19 , num. 2 , p. 555-562. DOI : 10.1021/acs.biomac.7b01664. Polymers from Nature and for Nature H. Sun ; H-A. Klok ; Z. Zhong
Biomacromolecules . 2018-06-01. Vol. 19 , num. 6 , p. 1697-1700. DOI : 10.1021/acs.biomac.8b00830. 2017 Journal Articles Microcomputed Tomography Technique for In Vivo Three-Dimensional Fat Tissue Volume Evaluation After Polymer Injection S. Berndt ; I. Konz ; D. Colin ; S. Germain ; B. Pittet-Cuenod et al.
Tissue Engineering Part C-Methods . 2017. Vol. 23 , num. 12 , p. 964-970. DOI : 10.1089/ten.tec.2017.0207. Caspofungin on ARGET-ATRP grafted PHEMA polymers: Enhancement and selectivity of prevention of attachment of Candida albicans T. D. Michl ; C. Giles ; P. Mocny ; K. Futrega ; M. R. Doran et al.
Biointerphases . 2017. Vol. 12 , num. 5 , p. 05G602. DOI : 10.1116/1.4986054. Cell-mediated delivery of synthetic nano- and microparticles funding M. Ayer ; H-A. Klok
Journal of Controlled Release . 2017. Vol. 259 , p. 92-104. DOI : 10.1016/j.jconrel.2017.01.048. Reversion of P-gp-Mediated Drug Resistance in Ovarian Carcinoma Cells with PHPMA-Zosuquidar Conjugates C. Battistella ; H-A. Klok
Biomacromolecules . 2017. Vol. 18 , num. 6 , p. 1855-1865. DOI : 10.1021/acs.biomac.7b00291. Site-Specific Polymer Attachment to HR2 Peptide Fusion Inhibitors against HIV-1 Decreases Binding Association Rates and Dissociation Rates Rather Than Binding Affinity M. Danial ; A. N. Stauffer ; F. R. Wurm ; M. J. Root ; H-A. Klok
Bioconjugate Chemistry . 2017. Vol. 28 , num. 3 , p. 701-712. DOI : 10.1021/acs.bioconjchem.6b00540. Peptide-Enhanced Selective Surface Deposition of Polymer-Based Fragrance Delivery Systems K. A. Guenay ; D. Benczedi ; A. Herrmann ; H-A. Klok
Advanced Functional Materials . 2017. Vol. 27 , num. 2 , p. 1603843. DOI : 10.1002/adfm.201603843. 2016 Journal Articles Influence of Block versus Random Monomer Distribution on the Cellular Uptake of Hydrophilic Copolymers J. Moraes ; R. Peltier ; G. Gody ; M. Blum ; S. Recalcati et al.
ACS Macro Letters . 2016. Vol. 5 , num. 12 , p. 1416-1420. DOI : 10.1021/acsmacrolett.6b00652. Degrafting of Poly(poly(ethylene glycol) methacrylate) Brushes from Planar and Spherical Silicon Substrates N. C. Ataman ; H-A. Klok
Macromolecules . 2016. Vol. 49 , num. 23 , p. 9035-9047. DOI : 10.1021/acs.macromol.6b01445. Impact of polymer-modified gold nanoparticles on brain endothelial cells: exclusion of endoplasmic reticulum stress as a potential risk factor L. Anspach ; R. E. Unger ; C. Brochhausen ; M. I. Gibson ; H-A. Klok et al.
Nanotoxicology . 2016. Vol. 10 , num. 9 , p. 1341-1350. DOI : 10.1080/17435390.2016.1214761. Swelling Behavior and Nanomechanical Properties of (Peptide-Modified) Poly(2-hydroxyethyl methacrylate) and Poly(poly(ethylene glycol) methacrylate) Brushes S. Desseaux ; J. P. Hinestrosa ; N. Schuwer ; B. S. Lokitz ; J. F. Ankner et al.
Macromolecules . 2016. Vol. 49 , num. 12 , p. 4609-4618. DOI : 10.1021/acs.macromol.6b00881. Click Chemistry in Biomaterials, Nanomedicine, and Drug Delivery K. S. Anseth ; H-A. Klok
Biomacromolecules . 2016. Vol. 17 , num. 1 , p. 1-3. DOI : 10.1021/acs.biomac.5b01660. Effects of Grafting Density and Film Thickness on the Adhesion of Staphylococcus epidermidis to Poly(2-hydroxy ethyl methacrylate) and Poly(poly(ethylene glycol)methacrylate) Brushes S-A. Ibanescu ; J. Nowakowska ; N. Khanna ; R. Landmann ; H-A. Klok
Macromolecular Bioscience . 2016. Vol. 16 , num. 5 , p. 676-685. DOI : 10.1002/mabi.201500335. Effect of Surface Charge on Surface-Initiated Atom Transfer Radical Polymerization from Cellulose Nanocrystals in Aqueous Media J. O. Zoppe ; X. Xu ; C. Kaenel ; P. Orsolini ; G. Siqueira et al.
Biomacromolecules . 2016. Vol. 17 , num. 4 , p. 1404-1413. DOI : 10.1021/acs.biomac.6b00011. Synthesis of cyclic peptide disulfide-PHPMA conjugates via sequential active ester aminolysis and CuAAC coupling K. A. Guenay ; H-A. Klok
Polymer Chemistry . 2016. Vol. 7 , num. 4 , p. 970-978. DOI : 10.1039/c5py01817j. 2015 Journal Articles Oligonucleotide Immobilization and Hybridization on Aldehyde-Functionalized Poly(2-hydroxyethyl methacrylate) Brushes T. Bilgic ; H-A. Klok
Biomacromolecules . 2015. Vol. 16 , num. 11 , p. 3657-3665. DOI : 10.1021/acs.biomac.5b01116. Avoiding compositional drift during the RAFT copolymerization of N-(2-hydroxypropyl)-methacrylamide and N-acryloxysuccinimide: towards uniform platforms for post-polymerization modification (vol 6, pg 3245, 2015) J. Moraes ; I-M. Simionca ; H. Ketari ; H-A. Klok
Polymer Chemistry . 2015. Vol. 6 , num. 42 , p. 7480-7483. DOI : 10.1039/c5py90156a. Shape-Persistent, Thermoresponsive Polypeptide Brushes Prepared by Vapor Deposition Surface-Initiated Ring-Opening Polymerization of alpha-Amino Acid N-Carboxyanhydrides Y. Shen ; S. Desseaux ; B. Aden ; B. S. Lokitz ; Z. Li et al.
Macromolecules . 2015. Vol. 48 , num. 8 , p. 2399-2406. DOI : 10.1021/acs.macromol.5b00017. Expanding the Polymer Mechanochemistry Toolbox through Surface-Initiated Polymerization H-A. Klok ; J. Genzer
ACS Macro Letters . 2015. Vol. 4 , num. 6 , p. 636-639. DOI : 10.1021/acsmacrolett.5b00295. Avoiding compositional drift during the RAFT copolymerization of N-(2-hydroxypropyl)methacrylamide and N-acryloxysuccinimide: towards uniform platforms for post-polymerization modification J. Moraes ; I-M. Simionca ; H. Ketari ; H-A. Klok
Polymer Chemistry . 2015. Vol. 6 , num. 17 , p. 3245-3251. DOI : 10.1039/c5py00253b. Fibroblast adhesion on ECM-derived peptide modified poly(2-hydroxyethyl methacrylate) brushes: Ligand co-presentation and 3D-localization S. Desseaux ; H-A. Klok
Biomaterials . 2015. Vol. 44 , p. 24-35. DOI : 10.1016/j.biomaterials.2014.12.011. Surface-initiated controlled radical polymerization enhanced DNA biosensing T. Bilgic ; H-A. Klok
European Polymer Journal . 2015. Vol. 62 , p. 281-293. DOI : 10.1016/j.eurpolymj.2014.07.037. Glucose Monitoring Using a Polymer Brush Modified Polypropylene Hollow Fiber-based Hydraulic Flow Sensor N. Fortin ; H-A. Klok
Acs Applied Materials & Interfaces . 2015. Vol. 7 , num. 8 , p. 4631-4640. DOI : 10.1021/am507927w. 2014 Journal Articles Maleimide-Functionalized Thiol Reactive Copolymer Brushes: Fabrication and Post-Polymerization Modification T. N. Gevrek ; T. Bilgic ; H-A. Klok ; A. Sanyal
Macromolecules . 2014. Vol. 47 , num. 22 , p. 7842-7851. DOI : 10.1021/ma5015098. Temperature-Controlled Masking/Unmasking of Cell-Adhesive Cues with Poly(ethylene glycol) Methacrylate Based Brushes S. Desseaux ; H-A. Klok
Biomacromolecules . 2014. Vol. 15 , num. 10 , p. 3859-3865. DOI : 10.1021/bm501233h. Glucose-Sensitive QCM-Sensors Via Direct Surface RAFT Polymerization C. Sugnaux ; H-A. Klok
Macromolecular Rapid Communications . 2014. Vol. 35 , num. 16 , p. 1402-1407. DOI : 10.1002/marc.201400217. Copolymerization of 2,2,3,3,4,4,4-heptafluorobutyl acrylate with butyl acrylate via RAFT polymerization B. P. Koiry ; H-A. Klok ; N. K. Singha
Journal Of Fluorine Chemistry . 2014. Vol. 165 , p. 109-115. DOI : 10.1016/j.jfluchem.2014.06.016. Polymer Brush Gradients Grafted from Plasma-Polymerized Surfaces B. R. Coad ; T. Bilgic ; H-A. Klok
Langmuir . 2014. Vol. 30 , num. 28 , p. 8357-8365. DOI : 10.1021/la501380m. Squaric acid mediated bioconjugation expanded to polymers prepared by ATRP T. Steinbach ; F. Wurm ; H-A. Klok
Polymer Chemistry . 2014. Vol. 5 , num. 13 , p. 4039-4047. DOI : 10.1039/c4py00168k. 2013 Journal Articles One-pot squaric acid diester mediated aqueous protein conjugation F. Wurm ; T. Steinbach ; H-A. Klok
Chemical Communications . 2013. Vol. 49 , num. 71 , p. 7815-7817. DOI : 10.1039/c3cc44039g. Postpolymerization Modification of Poly(glycidyl methacrylate) Brushes: An XPS Depth-Profiling Study R. Barbey ; V. Laporte ; S. Alnabulsi ; H-A. Klok
Macromolecules . 2013. Vol. 46 , num. 15 , p. 6151-6158. DOI : 10.1021/ma400819a. Aqueous Fabrication of pH-Gated, Polymer-Brush-Modified Alumina Hybrid Membranes C. Sugnaux ; L. Lavanant ; H-A. Klok
Langmuir . 2013. Vol. 29 , num. 24 , p. 7325-7333. DOI : 10.1021/la304949h. 2012 Journal Articles Squaric Acid Mediated Chemoselective PEGylation of Proteins: Reactivity of Single-Step-Activated alpha-Amino Poly(ethylene glycol)s C. Dingels ; F. Wurm ; M. Wagner ; H-A. Klok ; H. Frey
Chemistry-A European Journal . 2012. Vol. 18 , num. 52 , p. 16828-16835. DOI : 10.1002/chem.201200182. Osteoconductive surfaces generated from peptide functionalized poly(2-hydroxyethyl methacrylate-co-2-(methacryloyloxy)ethyl phosphate) brushes D. Paripovic ; H. Hall-Bozic ; H-A. Klok
Journal Of Materials Chemistry . 2012. Vol. 22 , num. 37 , p. 19570-19578. DOI : 10.1039/c2jm31568h. Site-Specific PEGylation of HR2 Peptides: Effects of PEG Conjugation Position and Chain Length on HIV-1 Membrane Fusion Inhibition and Proteolytic Degradation M. Danial ; V. Dulmen ; H. H. Tim ; J. Aleksandrowicz ; A. J. G. Poetgens et al.
Bioconjugate Chemistry . 2012. Vol. 23 , num. 8 , p. 1648-1660. DOI : 10.1021/bc3002248. Comparative Study on the In Vitro Cytotoxicity of Linear, Dendritic, and Hyperbranched Polylysine Analogues Z. Kadlecova ; L. Baldi ; D. Hacker ; F. M. Wurm ; H-A. Klok
Biomacromolecules . 2012. Vol. 13 , num. 10 , p. 3127-3137. DOI : 10.1021/bm300930j. Synthesis and post-polymerization modification of poly(pentafluorophenyl methacrylate) brushes K. A. Guenay ; N. Schuewer ; H-A. Klok
Polymer Chemistry . 2012. Vol. 3 , p. 2186-2192. DOI : 10.1039/c2py20162c. Hyperbranched Polylysine: A Versatile, Biodegradable Transfection Agent for the Production of Recombinant Proteins by Transient Gene Expression and the Transfection of Primary Cells Z. Kadlecova ; Y. Rajendra ; M. Matasci ; D. Hacker ; L. Baldi et al.
Macromolecular Bioscience . 2012. Vol. 12 , p. 794-804. DOI : 10.1002/mabi.201100519. Polyvalent Side Chain Peptide-Synthetic Polymer Conjugates as HIV-1 Entry Inhibitors M. Danial ; M. J. Root ; H-A. Klok
Biomacromolecules . 2012. Vol. 13 , p. 1438-1447. DOI : 10.1021/bm300150q. Poly(ethyleneimine)-Mediated Large-Scale Transient Gene Expression: Influence of Molecular Weight, Polydispersity and N-Propionyl Groups Z. Kadlecova ; S. Nallet ; D. L. Hacker ; L. Baldi ; H-A. Klok et al.
Macromolecular Bioscience . 2012. Vol. 12 , p. 628-636. DOI : 10.1002/mabi.201100404. Squaric Acid Mediated Synthesis and Biological Activity of a Library of Linear and Hyperbranched Poly(Glycerol)-Protein Conjugates F. Wurm ; C. Dingels ; H. Frey ; H-A. Klok
Biomacromolecules . 2012. Vol. 13 , p. 1161-1171. DOI : 10.1021/bm300103u. Functional, Hyperbranched Polyesters Via Baylis-Hillman Polymerization S. Ji ; B. Bruchmann ; F. Wurm ; H-A. Klok
Journal Of Polymer Science Part A-Polymer Chemistry . 2012. Vol. 50 , p. 25-34. DOI : 10.1002/pola.24954. 2011 Journal Articles Exploring the Scope of the Baylis-Hillman Reaction for the Synthesis of Side-Chain Functional Polyesters S. Ji ; B. Bruchmann ; H-A. Klok
Macromolecular Chemistry And Physics . 2011. Vol. 212 , p. 2612-2618. DOI : 10.1002/macp.201100482. Tuning the pH Sensitivity of Poly(methacrylic acid) Brushes N. Schuewer ; H-A. Klok
Langmuir . 2011. Vol. 27 , p. 4789-4796. DOI : 10.1021/la200347u. Aqueous solution self-assembly of polystyrene-b-poly(L-lysine) diblock oligomers H. Nuhn ; H-A. Klok
European Polymer Journal . 2011. Vol. 47 , p. 782-791. DOI : 10.1016/j.eurpolymj.2010.09.026. Improving the Stability in Aqueous Media of Polymer Brushes Grafted from Silicon Oxide Substrates by Surface-Initiated Atom Transfer Radical Polymerization D. Paripovic ; H-A. Klok
Macromolecular Chemistry And Physics . 2011. Vol. 212 , p. 950-958. DOI : 10.1002/macp.201000729. Sequentially Modified, Polymer-Stabilized Gold Nanoparticle Libraries: Convergent Synthesis and Aggregation Behavior M. I. Gibson ; M. Danial ; H-A. Klok
Acs Combinatorial Science . 2011. Vol. 13 , p. 286-297. DOI : 10.1021/co100099r. Arginine-specific protein modification using alpha-oxo-aldehyde functional polymers prepared by atom transfer radical polymerization M. A. Gauthier ; M. Ayer ; J. Kowal ; F. R. Wurm ; H-A. Klok
Polymer Chemistry . 2011. Vol. 2 , p. 1490-1498. DOI : 10.1039/c0py00422g. Synthesis of Side-Chain Functional Polyesters via Baylis-Hillman Polymerization S. Ji ; B. Bruchmann ; H-A. Klok
Macromolecules . 2011. Vol. 44 , p. 5218-5226. DOI : 10.1021/ma2006238.